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12-09 2023
Carbonyl Olefin Metathesis and Dehydrogenative Cyclization of...         Yunxiao Zhang, Jiaxin Wang, Youyuan Guo, Shanshan Liu, Xiao Shen.Angew. Chem. Int. Ed.（沈晓）Abstract：        The beauty of one-pot cascade reaction lies in the efficient disconnection and construction of several bonds in a single reaction flask, without the isolation of any intermediates. Herein, we report the first photo-induced thermal-promoted cascade reactions of readily available aromatic ...
12-03 2023
Selective C(sp3)–H arylation/alkylation of alkanes enabled b...                Long Zou,Siqi Xiang,Rui Sun & Qingquan Lu.Nature Communications.（陆庆全）Abstract：        We report a combination of electrocatalysis and photoredox catalysis to perform selective C(sp3)–H arylation/alkylation of alkanes, in which a binary catalytic system based on earth-abundant iron and nickel is applied. Reaction selectivity between two-component C(sp3)–H arylation and three-component ...
10-06 2023
Hydrogel-based Molecular Tension Fluorescence Microscopy for ...         Wenxu Wang,Wei Chen,Chaoyang Wu,Chen Zhang,Jingjing Feng,Pengxiang Liu,Yuru Hu,Hongyun Li,Feng Sun,Kai Jiang,Xinghua Zhang & Zheng Liu.Nature Methods.（刘郑）Abstract：        Extracellular matrix (ECM) rigidity serves as a crucial mechanical cue impacting diverse biological processes. However, understanding the molecular mechanisms of rigidity sensing has been limited by the spatial resolution ...
10-01 2023
Alkene 1,1-difunctionalizations via organometallic-radical re...         Dong Wu,Weiyu Kong,Yang Bao,Dengyang Zhao,Yuqiang Li &Guoyin Yin.Nature Catalysis.（阴国印、李玉强）Abstract：        Radical reactions play an important role in modern organic synthetic chemistry. The generation of carbon radicals from the homolytic cleavage of carbon–metal bonds has been widely studied as a fundamental step in organometallic chemistry. However, the implementation of this ...
09-16 2023
Boosting the Proton-coupled Electron Transfer via Fe-P Atomic...     Qiao Zhang, Hsin Jung Tsai, Fuhua Li, Zhiming Wei, Qinye He, Jie Ding, Yuhang Liu, Zih-Yi Lin, Xiaoju Yang, Zhaoyang Chen, Fangxin Hu, Xuan Yang, Qing Tang, Hong Bin Yang, Sung-Fu Hung, Yueming Zhai.Angew. Chem. Int. Ed.（翟月明）Abstract：        The  Single-atom catalysts exhibit superior CO2-to-CO catalytic activity, but poor kinetics of proton-coupled electron transfer (PCET) steps still limit ...
09-08 2023
Elucidating the Underlying Reactivities of Alternating Curren...     Qiongqiong Wan, Kaixiang Chen, Xin Dong, Xianqin Ruan, Prof. Hong Yi, Prof. Suming Chen.Angew. Chem. Int. Ed.（陈素明、易红）Abstract：        The Alternating current (AC) electrolysis is an emerging field in synthetic chemistry, however its mechanistic studies are challenged by the effective characterization of the elusive intermediate processes. Herein, we develop an operando electrochemical ...
07-25 2023
Single Nanoparticle-Based Nanomachining for Fabrication of Un...     Longfei Miao, Bintong Huang, Hui Fang, Jia Chai, Ze Liu, Yueming Zhai.Advanced Materials（翟月明）Abstract：        The structure of nanomaterials and nanodevices determines their functionality and applications. A single uniform nanochannel with a high aspect ratio is an attractive structure due to its unique rigid structures, easy preparation and diverse pore structures that hold significant promising ...
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